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On the Temperature Dependence of Molecular Line Shapes Due to Linearly Coupled Phonon Bands
Temperature Dependent Molecular Line Shapes Linearly Coupled Phonon Bands
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2014/9/24
Simple closed-form expressions of line-shape functions are derived for models of a two-level chromophore linearly coupled to harmonic oscillator baths on the basis of an accurate approximation for the...
Molecular Pulses: Population inversion with positively chirped short pulses
Molecular Pulses Population inversion positively chirped short pulses
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2014/9/24
Detailed theoretical analysis and numerical simulation indicate that nearly complete electronic population inversion of molecular systems can be achieved with intense positively chirped broadband lase...
Chirped pulse enhancement of multiphoton absorption in molecular iodine
Chirped pulse enhancement multiphoton absorption molecular iodine
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2014/9/24
Chirp effects on three photon absorption yields in I2 vapor are investigated using femtosecond pulses with center wavelengths in the region 550–600 nm. Enhancements of as much as a factor of 3 are obs...